Figure 1 shows a schematic diagram of the CME package (264 mm length x 330 mm width x 570 mm height), which weighs about 25 kg. The main components are a drier, a pump, solenoid valves, a flow controller, a pressure controller, NDIR analyzer (LICOR, LI-840), two standard gas cylinders, and a programmable controller/datalogger device (Figure 2). Air samples are drawn by a diaphragm pump from the intake port mounted on the air conditioning duct and then introduced into the analyzer. In the upstream of the pump, a drier tube packed with CO2-saturated magnesium perchlorate is used to remove water vapor. The flow rate of the sampled air into the NDIR cell is kept constant at 150 standard cc per minute (sccm) by a mass flow controller. In addition, the absolute pressure of the sampled air in the NDIR cell is maintained at 0.110 MPa by an auto pressure controller to avoid signal drift in the NDIR associated with changes in cabin pressure.
Navigation data received by the controller/datalogger device include date, time, pressure altitude, radio altitude, latitude, longitude, ground speed, static air temperature, and wind direction and velocity. In order to avoid sampling of heaviliy polluted air (high CO2 and H2O) in the lower layers of the atmosphere, air sampling does not start until the radio altitude registers 2000 feet during the ascent, and stops at 2000 feet during the descent. All of the data from the aircraft data system, the NDIR signal, flow rate, cell pressure and supplied air pressure measured by pressure sensor 1 are recorded every 10 seconds during the ascent and descent and every 1 minute during the level flight. The time interval of 10 seconds corresponds to about 100m in altitude, while that of 1 minute corresponds to 10-20 km in the horizontal. The measurement precision is estimated to be 0.1 ppm (one standard deviation) when using 10-second averaged data. Thus, CME enables us to resolve the fine structures of the atmospheric CO2 distribution from all of the flights (Machida et al. 2008).
Figure 2. Photo of CME. The surface panels are detached.
Latitudinal distributions of CO2 measured by CME in the upper troposphere between Sydney and Narita are compared in Figure 3 with those obtained by ASE during the December 8, 2005 flight. Both data are in a good agreement, i.e. within ±0.2ppm. Data from other flights carrying ASE and CME show likewise good agreements. Analytical precision and accuracy are relatively better for ASE since flask samples are analyzed by a LI-6252 (LICOR) in our laboratory under controlled conditions. Therefore, the data agreement indicates a high reliability in CO2 measurements by a small NDIR inside the CME.
Figure 3. Latitudinal distributions of CO2 mixing ratio in the upper troposphere measured on December 8, 2005 by CME and ASE. The green line indicates flight altitude.
Figure 4 shows vertical CO2 distributions obtained over Narita, Japan (NRT) and Jakarta, Indonesia (CGK) on 5–8 November 2005. High CO2 values near the surface reflect CO2 contaminated by human activities around the airport. Vertical profiles in the free troposphere are tightly bound over both airports, indicating high reproducibility of CME observation. The vertical gradient with higher CO2 mixing ratios at the lower altitudes over NRT (Figure 4a) is caused by CO2 release from land vegetation and fossil fuel use in this area. On the other hand, relatively constant CO2 with height over CGK is reflective of the wide tropical region where net surface CO2 emissions are weak and vertical air mixing is efficient; these observation results are similar to results from a previous aircraft observation campaign (Machida et al. 2003).
Figure 4. Vertical distributions of CO2 mixing ratio observed on 5-8 November 2005 over Narita, Japan (a) and Jakarta, Indonesia (b).
Distribution of CO2 in the atmosphere varies with meteorology. Figure 5 (Click to view) illustrates an example of how CO2 distribution at the cruising altitude (about 10 km) changes during a month together with when and where our aircraft measured CO2. The CO2 distirbutions were computed by an atmospheric transport model (Niwa et al. 2012)
Figure 5. Animation of atmospheric CO2 with CME tracks at about 10 km.
After 10 years of CME measurements, we obtained > 7 million CO2 data points from > 12 thousand flights. In particular, we have the highest data density over the Asia-Pacific region. The numerous data enabled us seasonal climatology of CO2 distribution well visualized horizontally and vertically over Asia (Figure 6).
Figure 6. Animation of monthly atmospheric CO2 distributions over Asia measured by CME (upper panel and pillers). The number at right-top shows month. The colors at the lower panel indicate monthly biospheric fluxes (Red—source, Blue—sink) estimated by using an atmospheric transport model (Niwa et al. 2012). Produced from figures in Umezawa et al. 2018.
Last update: 10 May 2019
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